Watermelons are among the most musically gruesome
A simulated bell pepper made of Styrofoam, definitely never alive … but hollow, with a thin but relatively rigid outer shell, would make a very similar sound to an actual pepper when cracked open, though admittedly a bit of wetness would add a useful layer.
The magic comes from the combination of a rigid layer encasing a hollow or at least soft interior. The internal resonance that happens when the rigid layer is cracked is a big part of the appeal, and the sonically delicious icing on the cake is that the resonant frequency changes dynamically as the shape of the cavity changes in the course of the destruction.
Another factor that favors these kinds of vegetables over a carrot, for example, is duration. A snap of only a few milliseconds in length, what you get when you break a carrot, is almost never going to be as interesting as a more elongated rip or tear that lasts more like a second.
That’s why peppers (the bigger and more hollow the better), and celery, and cabbage, and watermelons are among the most musically gruesome of veggies.
And why they’re so good at simulating and creatively exaggerating the fracturing sound of other objects with hard shells and soft insides, like bones and craniums.
Hollow things in general tend to make sounds interesting to humans, which is why so many musical instruments are comprised of at least one hollow component.